Papers - TEZUKA YASUHISA
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Pressure-dependent electronic structure of the A-site ordered perovskite CaCu3Ti4O12 via x-ray Raman scattering
Yasuhisa Tezuka, Hojun Im, Takao Watanabe, Hirofumi Ishii, Nozomu Hiraoka, Yoichi Ishiwata, Hitoshi Yamaoka
Physical Review B 109 ( 3 ) 035132-1 - 035132-8 2024.1
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Temperature dependence of electronic structure on the ferroelectric phase transition of BaTiO3
Y. Tezuka, S. Nozawa, N. Nakajima, and T. Iwazumi
Phys. Rev. B 104 ( 23 ) 235148-1 - 235148-7 2021.12
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Polarization dependent Cu 2p resonant X-ray Raman Scattering of CaCu3Ti4O12
Y. Tezuka, M. Shimamura, H. Im, and T. Watanabe
Photon Factory Activity Report 2023 41 158 - 158 2024.7
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Atomic and Electronic Structures on a Mordenite Zeolite
Hosokawa Shinya, Sato Hitoshi, Tezuka Yasuhisa, Adachi Jun-ichi, Kimura Koji, Hayashi Koichi, Kohara Shinji, Tajiri Hiroo, Kobayashi Kentaro, Koura Akihide, Shimojo Fuyuki
e-Journal of Surface Science and Nanotechnology 22 ( 1 ) 25 - 31 2023.9
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Atomic and electronic structures of an Ag-containing 4A zeolite
Shinya Hosokawa, Kentaro Kobayashi, Akihide Koura, Fuyuki Shimojo, Yasuhisa Tezuka, Jun ichi Adachi, Yohei Onodera, Shinji Kohara, Hiroo Tajiri, Anand Chokkalingam, Toru Wakihara
Microporous and Mesoporous Materials 359 112662-1 - 112662-8 2023.9
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Temperature Dependent Electronic Structure of A-site Ordered Perovskite CaCu3Ti4O12
M. Shimamura, H.J. Im, T. Watanabe, S. Nozawa, N. Nakajima, T. Iwazumi, and Y. Tezuka
Photon Factory Activity Report 2022 40 200 - 200 2023.7
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Temperature dependence of resonant X-ray Raman scattering of SrTiO3.
Y.Tezuka, M.Shimamura, S.Nozawa, and T.Iwazumi
Photon Factory Activity Report 2021 38 174 - 174 2022.7
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Correlation between ferromagnetism and dopant 3d metal-oxygen hybridized state lying at the bottom of conduction band in ZnO-based diluted magnetic semiconductor system
T. Tsukahara, S. An, S. Otsuru, Y. Tezuka, S. Nozawa, J. Adachi, K. Akashi, Y. Inagaki, T. Kawae, H. Ishii, Y.F. Liao, T. Kida, S. Suehiro, M. Nantoh, K. Ishibashi, and Y. Ishiwata
J. Appl. Phys. 130 ( 24 ) 24390-1 - 24390-7 2021.12
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Elaboration of near-valence band defect states leading deterioration of ambipolar operation in SnO thin-film transistors
M. Minohara, S. Asanuma, H. Asai, Y. Dobashi, A. Samizo, Y. Tezuka, K. Ozawa, K. Mase, I. Hase, N. Kikuchi, and Y. Aiura
Nano Select 2021 ( 6 ) 1 - 9 2021.11
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Temperature Dependent Local Structure of A-Site Ordered Perovskite CaCu3Ti4O12 Measured by X-Ray Fluorescence Holography
M. Asari, H.J. Im, T. Watanabe, N. Happo, K. Kimura, K. Hayasi, S. Hosokawa, and Y. Tezuka
Photon Factory Activity Report 2020 38 177 - 177 2021.7
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O 2p partial density of states in Sn b-zeolite by soft x-ray emission spectroscopy
S. Hosokawa, Y. Tezuka and T. Wakihara
Photon Factory Activity Report 2020 38 114 - 114 2021.7
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Polarization Dependent Ti 2p Resonant X-Ray Raman Scattering Study of CaCu3Ti4O12
R. Kato1, H. Im, T. Watanabe, N. Nakajima, and Y. Tezuka
Photon Factory Activity Report 2020 38 178 - 178 2021.7
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Partial density of states in functional zeolite by soft x-ray emission spectroscopy
S. Hosokawa, H. Sato, Y. Tezuka
Photon Factory Activity Report 2019 (KEK) #37 47 - 47 2020.7
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Temperature dependent electronic structure of SrTiO3 by means of resonant X-ray Raman scattering
M. Takahashi, S. Nozawa, N. Nakajima, T. Iwazumi, Y. Tezuka
Photon Factory Activity Report 2019 (KEK) #37 204 - 204 2020.7
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Local Structure Study of A-site Ordered Perovskite CaCu3Ti4O12 by means of X-ray Fluorescence Holography
H. Kamide, H.J. Im, T. Watanabe, N. Happo, K. Kimura, K. Hayashi, S. Hosokawa, and Y. Tezuka
Photon Factory Activity Report 2018 (KEK) #36 191 - 191 2019.7
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In-gap state generated by La-on-Sr substitutional defects within the bulk of SrTiO3
Yoshihiro Aiura, Kenichi Ozawa, Yasuhisa Tezuka, Makoto Minohara, Akane Samizo, Kyoko Bando, Hiroshi Kumigashira, Kazuhiko Mase
PHYSICAL CHEMISTRY CHEMICAL PHYSICS 21 ( 27 ) 14646 - 14653 2019.7
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Temperature Dependent O K Resonant X-ray Emission Spectra of CaCu3Ti4O12
Y. Tezuka, H. Kamide, H.J. Im, T. Watanabe, and N. Nakajima
Photon Factory Activity Report 2017 (KEK) #35 283 - 283 2018.7
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La0.05Sr0.95TiO3のX線発光分光 X-Ray Emission Spectroscopy on La0.05Sr0.95TiO3
相浦義弘, 手塚泰久, 上出晴輝, 小澤健一, 足立純一, 間瀬一彦
Photon Factory Activity Report 2018 (KEK) #35 88 - 88 2018.7
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Polarization-Dependent Ti 2p-Resonant X-ray Raman Scattering from Ti2O3
Y. Tezuka, N. Nakajima, J. Adachi, O. Morimoto, H. Sato, and T. Uozumi
Journal of Physical Society of Japan 86 124713-1 - 124713-5 2017.11
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Temperature Dependent Electronic Structure Study of CaCu3Ti4O12 by Means of X-Ray Raman Scattering
K. Nishiyama, S. Nakamoto, H. Im, T. Watanabe, S. Nozawa, N. Nakajima, T. Iwazumi, and Y. Tezuka
Photon Factory Activity Report 2016 (KEK) #34-B 286 - 286 2017.7
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Electronic Structure Study of CaCu3Ti4O12 by means of X-ray Raman Scattering
Y. Tezuka, Y. Yokouchi, S. Sasaki, S. Nakamoto, K. Nishiyama, M. Mikami, H.J. Im, T. Watanabe, S. Nozawa, N. Nakajima, and T. Iwazumi
Journal of Electron Spectroscopy and Related Phenomena 220 114 - 117 2017.4
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Electronic Structure Study of CaCu3Ti4O12 by means of Soft X-ray Raman Scattering
S. Nakamoto, K Nishiyama, H. Im, T. Watanabe, N. Nakajima, and Y. Tezuka
Photon Factory Activity Report 2015 (KEK) #33-B 378 - 378 2016.7
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Electronic Structure Study of CaCu3Ti4O12 by means of X-ray Raman Scattering
Y. Yokouchi, M. Mikami, H. Im, T. Watanabe, S. Nozawa, N. Nakajima, T. Iwazumi, Y. Tezuka
Photon Factory Activity Report 2014 (KEK) 32 195 - 195 2015.12
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Electronic Structure Study of nano-particle Anatase (TiO2) by means of X-ray Raman Scattering
Y. Tezuka, S. Nakamoto, Y. Yokouchi, M. Mikami, S. Nozawa, T. Iwazumi, and Y. Ishiwata
Photon Factory Activity Report 2014 (KEK) 32 194 - 194 2015.12
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Time-Resolved X-ray Absorption Spectroscopy of BaTiO3 Under Pulsed Electric Field
A. Sano, N. Nakajima, J. Adachi, Y. Niwa, and Y. Tezuka
Photon Factory Activity Report 2014 (KEK) 32 177 - 177 2015.12
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Impurity-Induced First-order Phase Transitions in Highly Crystalline V2O3 Nanocrystals
Y. Ishiwata, E. Takahashi, K. Akashi, M. Imamura, J. Azuma, K. Takahashi, M. Kamada, H. Ishii, Y.-F. Liao, Y. Tezuka, Y. Inagaki, T. Kawae, D. Nishio-Hamane, M. Nantoh, K. Ishibashi and T. Kida
Advanced Materials Interfaces 2 1500132-1 - 1500132-6 2015.8
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Oxygen 2p Partial Density of States and Bond Angles around O Atoms in SiO2 Glass
S. Hosokawa, H. Sato, K. Mimura, Y. Tezuka, D. Fukunaga, Y. Matsuzaki, and F. Shimojo
Journal of Physical Society of Japan 84 024605-1 - 024605-6 2015.1
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ノンドープ、CoドープおよびVドープTiO2ナノ粒子の軟X 線発光分光
石渡洋一, 高橋栄光, 赤司健太, 手塚泰久
Photon Factory Activity Report 2013 (KEK) #31-B 555 - 555 2015.1
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Electronic Structure Study of Anatase (TiO2) under UV irradiation by means of X-ray Raman Scattering
M. Mikami, R. Oura, Y. Sasaki, S. Nozawa, T. Iwazumi, Y. Ishiwata, K. Ozawa, M. Emori, H. Sakama, Y. Tezuka
Photon Factory Activity Report 2013 (KEK) #31-B 325 - 325 2015.1
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Oxygen 2p partial density of states in a typical oxide glass B2O3
S. Hosokawa, H. Sato, K. Mimura, Y. Tezuka, D. Fukunaga, K. Shimamura1, and F. Shimojo
Photon Factory Activity Report 2013 (KEK) #31-B 154 - 154 2015.1
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Oxygen 2p Partial Density of States and Bond Angles around O Atoms in SiO2 Glass
S. Hosokawa, H. Sato, K. Mimura, Y. Tezuka, D. Fukunaga, Y. Matsuzaki, and F. Shimojo
Journal of Physical Society of Japan 84 024605-1 - 024605-6 2015.1
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Electronic Structure Study of CaCu3Ti4O12 by means of X-ray Raman Scattering.
Y. Tezuka, M. Mikami, Y. Yokouchi, H. Im, T. Watanabe, S. Nozawa, N. Nakajima, T. Iwazumi
Photon Factory Activity Report 2013 (KEK) #31-B 323 - 323 2014.12
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Oxygen 2p Partial Density of States in a Typical Oxide Glass B2O3
S. Hosokawa, H. Sato, K. Mimura, Y. Tezuka, D. Fukunaga, K. Shimamura, and F. Shimojo
Journal of Physical Society of Japan 83 114601-1 - 114601-6 2014.10
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X-ray Raman Scattering Study of Structural Phase Transition of Ferroelectric BaTiO3
R. Oura, Y. Sasaki, M. Mikami, N. Nakajima, S. Nozawa, T. Iwazumi and Y. Tezuka
Photon Factory Activity Report 2012 (KEK) #30-B 120 - 120 2014.1
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Core Excitations in Resonant X-ray Raman Scattering of Titanium Oxides: An Approach to Studying Electronic Structures
Y. Tezuka, T. Sasaki, Y. Fujita, T. Iwamoto, H. Osawa, S. Nozawa, N. Nakajima, H. Sato, and T. Iwazumi
Journal of Physical Society of Japan 83 014707-1 - 014707-4 2014.1
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UV-Induced Change in the Electronic Structure of SrTiO3 at Low Temperature Probed by Resonant X-ray Emission Spectroscopy
S. Kawakami, N. Nakajima, T. Takigawa, M. Nakatake, H. Maruyama, Y. Tezuka, and T. Iwazumi
Journal of Physical Society of Japan 82 053701-1 - 053701-4 2013.4
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Electric-Field-Induced Insulator–Metal Transition in Ca2RuO4 Probed by X-ray Absorption and Emission Spectroscopy
M. Sakaki, N. Nakajima, F. Nakamura, Y. Tezuka, and T. Suzuki
Journal of Physical Society of Japan 82 014707-1 - 014707-9 2013.4
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O 2p partial density of states and local structures in oxide glasses
S. Hosokawa, H. Sato, K. Mimura, Y. Tezuka
Photon Factory Activity Report 2011 (KEK) #29-B 148 - 148 2013.1
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Electronic Structure and Local Atomic Arrangement in 2-dimensional Quasicrystals Al-Co-Ni
K. Soda, M. Inukai, Y.-G. So, K. Edagawa, Y. Yokoyama,Y. Tezuka, O. Morimoto
Photon Factory Activity Report 2011 (KEK) #29-B 133 - 138 2013.1
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Electronic Structure of Anatase (TiO2) by means of X-ray Raman Scattering.
Y. Tezuka, S. Jin, R. Oura, Y. Sasaki, S. Nozawa
Photon Factory Activity Report 2011 (KEK) #29-B 138 - 138 2013.1
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Enhancement of dielectric constant of BaTiO3 nanoparticles studied by resonant x-ray emission spectroscopy
N. Nakajima, M. Oki, Y. Isohama, H. Maruyama, Y. Tezuka, K. Ishiji, T. Iwazumi, and K. Okada
Physical Review B 86 224114-1 - 224114-4 2012.12
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Spontaneous uniaxial strain and disappearance of the metal-insulator transition in monodisperse V2O3 nanocrystals
Y. Ishiwata, S. Suehiro, T. Kida, H. Ishii, Y. Tezuka, H. Oosato, E. Watanabe, D. Tsuya, Y. Inagaki, T. Kawae, M. Nantoh, K. Ishibashi
Physical Review B 86 ( 3 ) 035449-1 - 035449-5 2012.7
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Anisotropic Electronic Structure of Ferroelectric BaTiO3 Measured by X-ray Raman Scattering.
Y. Tezuka, N. Nakajima, H. Osawa, S. Nozawa, T. Iwazumi, Y. Isozumi
Photon Factory Activity Report 2010 (KEK) #28-B 92 - 92 2012.1
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Detailed Measurement of Ti 2p Resonant X-ray Raman Scattering of Ti2O3 and its Polarization Dependence.
Y. Tezuka, T. Shinoya, H. Soyama, S. Nakagawa, O. Morimoto
Photon Factory Activity Report 2010 (KEK) #28-B 105 - 105 2012.1
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Metal-insulator transition sustained by Cr-doping in V2O3 nanocrystals
Y. Ishiwata, T. Shiraishi, N. Ito, S. Suehiro, T. Kida, H. Ishii, Y. Tezuka, Y. Inagaki, T. Kawae, H. Oosato, E. Watanabe, D. Tsuya, M. Nantoh, K. Ishibashi
App. Phys. Lett. 100 043103-1 - 043103-3 2012.1
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Detailed measurement of Ti 2p resonant X-ray Raman scattering of TiO2 and its polarization dependence measurements
Y. Tezuka, N. Nakajima, O. Morimoto
J. Elec. Spec. Relat. Phenom. 184 216 - 219 2011.4
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Tetragonal–cubic phase transition in BaTiO3 probed by resonant X-ray emission spectroscopy
Y. Isohama, N. Nakajima, H. Maruyama, Y. Tezuka, T. Iwazumi
J. Elec. Spec. Relat. Phenom. 184 207 - 209 2011.4
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Polarization-Dependent Ti K X-Ray Absorption and Emission Studies of Ti2O3 Single Crystal
H. Satoa, H. Maso, Y. Utsumi, H. Kurihara, Y. Mukaegawa, Y. Tezuka, T. Iwazumi, F. Igae, M. Tsubota, H. Namatame, M. Taniguchi
J. Elec. Spec. Relat. Phenom. 184 184 - 187 2011.4
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V 3d-2p soft x-ray emission spectrum of CuV2S4
Y. Taguchi, T. Mizoroki, K. Kodama, K. Mimura, H. Ishibashi, O. Morimoto. Y. Tezuka
Photon Factory Activity Report 2009 #27 Part B 27 89 - 89 2010.12
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Contour Plot of Soft X-ray Raman Scattering of Ti2O3
Y. Tezuka, T. Shinoya, H. Soyama, S. Nakagawa, N. Nakajima, O. Morimoto
Photon Factory Activity Report 2009 #27 Part B 27 100 - 100 2010.12
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X-ray Spectroscopic Study on Photoluminescence Properties of Red Phosphor SrTiO3:Pr3+,Al.
N. NAKAJIMA, Y. TEZUKA, et al.
Japanese Journal of Applied Physics 49 09ME04/1 - 09ME04/4 2010.9
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Unusual low-temperature phase in VO2 nanoparticles.
Y. ISHIWATA, Y. TEZUKA, et al.
Physical Revew B 82 115404/1 - 115404/7 2010.9
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Spectroscopic study on chemical ordering of transition metals in decagonal Al-Co-Ni and Al-Co-Cu quasicrystals.
M. INUKAI, Y. TEZUKA, et al.
Journal of Physics: Conference Series 226 012010/1 - 012010/6 2010.9
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Metal-insulator transition for V2O3 powder observed using a soft x-ray emission spectroscopy.
Y. ISHIWATA, Y. TEZUKA, et al.
Journal of the Physical Society of Japan 79 054712/1 - 054712/3 2010.5
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Soft x-ray absorption and emission study on anisotropic electronic structure of MoO3
H. SATO, Y. TEZUKA, et al.
Journal of Electron Spectroscopy and Related Phenomena 181 211 - 214 2010.2
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The mechanism of Al donor defects in (Zn, Co)O:Al: a view from resonant x-ray spectroscopies
K.J. Zhou, Y. Tezuka, et al.
Journal of Physics: Condensed Matter 21 495502/1 - 495502/7 2009.12
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Polarization Dependent X-ray Raman Scattering of TiO2(100)
Y. Tezuka, N. Nakajima, O. Morimoto
Photon Factory Activity Report 2008 (KEK) 26-B 86 - 86 2009.11
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Polarization-Dependent Ti K X-ray Absorption and Emission Studies of Ti2O3 Single Crystal
H. Maso, H. Kurihara, Y. Mukaegawa, Y. Utsumi, H. Sato, Y. Tezuka, T. Iwazumi, F. Iga, M. Tsubota, H. Namatame, M. Taniguchi
Photon Factory Activity Report 2007 (KEK) 25-B 93 - 93 2008.11
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Soft X-ray Raman Scattering of BaTiO3(100) by Means of Improved Spectrometer at BL-2c
Y. TEZUKA, N. Nakajima, O. Morimoto
Photon Factory Activity Report 2007 (KEK) 25-B 96 - 96 2008.11
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Polarization Dependent X-ray Raman Scattering of TiO2(100)
Y. TEZUKA, T. IWAMOTO, H. OSAWA, S. NOZAWA, T. IWAZUMI, Y. ISOZUMI
Photon Factory Activity Report 2007 (KEK) 25-B 76 - 76 2008.11
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強誘電体BaTiO3の共鳴X線ラマン散乱の研究
手塚泰久
Annual Report of The Murata Science Foundation 21 633 - 633 2007.12
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Soft X-Ray Absorption and Emission Study on Anisotropy of Electronic Structure of MoO3
Y. Mukaegawa, H. Sato, H. Kurihara, H. Maso, Y. Tezuka, O. Morimoto, H. Negishi, S. Negishi, H. Namatame, M. Taniguchi
Photon Factory Activity Report 2006 (KEK) 24-B 80 - 80 2007.11
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Ti 2p Soft X-ray Emission Spectroscopy of Ti2O3
H. Sato, K. Tsuji, K. Yoshikawa, Y. Tezuka, S. Nishimoto, M. Higashi, F. Iga, M. Tsubota, M. Taniguchi
Photon Factory Activity Report 2006 (KEK) 24-B 70 - 70 2007.11
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Resonant X-ray Raman Scattering Study of TiO2
Y. Tezuka, T. Sasaki, Y. Fujita, T. Iwamoto, H. Osawa, T. Iwazumi, Y. Isozumi
Photon Factory Activity Report 2006 (KEK) 24-B 69 - 69 2007.11
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Particle-Size Dependence of Resonant X-Rray Emission Spectroscopy in BaTiO3
N. Nnakajima, M. Oki, N. Ishimatsu, H. Maruyama, Y. Tezuka, K. Ishiji, T. Iwazumi
Photon Factory Activity Report 2006 (KEK) 24-B 68 - 68 2007.11
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Ab initio x-ray absorption near-edge structure study of Ti K-edge in rutile
J Chaboy, N Nakajima, Y Tezuka
Journal of Physics: Condensed Matter 19 266206-1 - 266206-9 2007.7
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Energy Distribution of Co and Ni 3d states of Decagonal Quasicrystal Al72Co16Ni12
M. Inukai, K. Soda, S. Ota, H. Miyazaki, T. Suzuki, M. Kato, S. Yagi, Y. Tezuka, Y. Yokoyama
Philosophical Magazine 87 3003 - 3010 2007.7
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Electronic structure of Pd42.5Ni7.5Cu30P20, an excellent bulk metallic glass former: Comparison to the Pd40Ni40P20 reference glass
S. Hosokawa, H. Sato, N. Happo, K. Mimura, Y. Tezuka, T. Ichitsubo, E. Matsubara, N. Nishiyama
Acta Materialia 55 3413 - 3419 2007.3
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Ti 2p soft X-ray emission spectroscopy of Ti2O3
H. Sato, K. Tsuji, K. Yoshikawa, Y. Tezuka, S. Nishimoto, M. Higashi,
Journal of Electron Spectroscopy and Related Phenomena 156-158 365 - 368 2007.1
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Soft X-ray emission study of Pd–Ni–Cu–P bulk metallic glass
S. Hosokawa,., H. Sato, K. Mimura, N. Happo, Y. Tezuka, T. Ichitsubo, E. Matsubara, N. Nishiyama
Journal of Electron Spectroscopy and Related Phenomena 156-158 3413 - 3419 2007.1
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Soft X-ray emission study of BaTiO3 nanoparticles
M. Oki, N. Nakajima, H. Maruyama, Y. Tezuka, T. Toda
Photon Factory Activity Report 2005 (KEK) 23-B 79 - 79 2006.11
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Resonant Soft X-ray Raman Scattering of BaTiO3
Y. Tezuka, T. Sasaki, Y. Fujita, M. Oki, N. Nakajima
Photon Factory Activity Report 2005 (KEK) 23-B 100 - 100 2006.11
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Co and Ni 3d States of Al72Ni12Co16 Quasicrystal
M. Inukai, H. Miyazaki, S. Ota, T. Suzuki, M. Kato, S. Yagi, K. Soda, Y. Tezuka, Y. Yokoyama
Photon Factory Activity Report 2005 (KEK) 23-B 84 - 84 2006.11
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X-ray Raman Scattering of Ti-Oxides Observed below Ti K Absorption Edge
Y. Tezuka, T. Sasaki, Y. Fujita, H. Osawa, T. Iwazumi, Y. Isozumi
Photon Factory Activity Report 2005 (KEK) 23-B 82 - 82 2006.11
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Polarization dependence of soft-x-ray Raman scattering of Ti2O3
Y. Tezuka, T. Maeda, Y. Harada, T. Takeuchi, H. Osawa, S. Shin, N. Nakajima
Photon Factory Activity Report 2004 (KEK) 22-B 111 - 111 2005.11
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Soft X-ray fluorescence spectroscopy of FexCo1-xSi
N. Nakajima, T. Maeda, K. Seong, N. Ishimatsu, Y. Tezuka, Y. Enta, H. Maruyama
Photon Factory Activity Report 2004 (KEK) 22-B 102 - 102 2005.11
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X-ray spectroscopy study on the electronic structure of hole-doped
E. Kabasawa, J. Nakamura, T. Morimoto, N. Yamada, K. Kuroki, H. Yamazaki, K. Okada, K. Oka, Y. Tezuka, J. D. Denlinger, R. C. C. Perera
Journal of Electron Spectroscopy and Related Phenomena 148 65 - 72 2005.4
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Observation of Conduction Band Satellite of Ni Metal by 3p-3d Resonant Inverse Photoemission Study
Y. Tezuka, K. Kanai, H. Ishii, S. Shin, S. Nozawa, A. Tanaka, T. Jo
Physical Review B, Condensed Matter and Materials Physics 70 193107-1 - 193107-4 2004.11
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Unoccupied Electronic State of SrTi1-xNbxO3 Observed by Inverse-Photoemission Spectroscopy
T. Higuchi, Y. Tezuka, T. Hattori, S. Yamaguchi, S. Shin, T. Tsukamoto
Japanese Journal of Applied Physics 43 ( 11A ) 7623 - 7624 2004.11
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Resonant inverse photoemission spectroscopy in soft X-ray region
Y. Tezuka, S. Shin
Journal of Electron Spectroscopy and Related Phenomena 136 151 - 160 2004.5